New Frontiers in Applications of Photocatalysis Processes

A special issue of Applied Sciences (ISSN 2076-3417). This special issue belongs to the section "Environmental Sciences".

Deadline for manuscript submissions: closed (20 December 2021) | Viewed by 1914

Special Issue Editor


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Guest Editor
College of Environmental Science and Engineering, North China Electric Power University, Beijing 102206, China
Interests: photocatalytic selective oxidation; heavy metal ions removal; surface modification; heterogeneous catalysis; solar energy utilization

Special Issue Information

Dear Colleagues,

Photocatalysis has been widely studied in the past few decades with respect to the degradation of pollutants, water splitting, CO2 reduction, N2 fixation and the recently emerged organic conversion/reforming. Although various types of photocatalysts/cocatalysts have been designed, achieving enhanced performance is usually based on the complicated or high-cost preparation of the catalysts, as well as corrosion/deactivation of the photocatalysts after long-time operation, which largely limits the practical application of photocatalysis to achieve efficient solar energy conversion and utilization. Thus, for this Special Issue, the purpose is to disseminate information and research results to inspire more study on practical and applicable photocatalysis systems. Particular attention will be given to those works that introduce stable and efficient photocatalysts, non-precious cocatalysts and new photocatalytic reactions that could take the place of thermo-catalytic processes with high efficiency and selectivity under mild reaction conditions.

Prof. Dr. Guixia Zhao
Guest Editor

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Keywords

  • photocatalysis
  • cocatalysts

Published Papers (1 paper)

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Research

12 pages, 2012 KiB  
Article
Effective Photocatalytic Hydrogen Evolution Using Covalent Triazine Framework-Derived Carbon Nitride Nanofiber Containing Carbon Vacancies for Visible-Light-Driven
by Liangjing Zhang, Aiwu Wang, Mei Zhang, Zhengyuan Jin, Huan Yi and Meng Wang
Appl. Sci. 2021, 11(16), 7222; https://0-doi-org.brum.beds.ac.uk/10.3390/app11167222 - 05 Aug 2021
Cited by 2 | Viewed by 1558
Abstract
In this study, a novel fibrous carbon nitride (FCN) was prepared from laminated covalent triazine framework (CTF) via pyrolysis, using functionalized 2,5-thiophenedicarboxylic acid and melamine as the precursors. A carbon vacancy was produced by two-step calcination in argon and air atmospheres. These carbon [...] Read more.
In this study, a novel fibrous carbon nitride (FCN) was prepared from laminated covalent triazine framework (CTF) via pyrolysis, using functionalized 2,5-thiophenedicarboxylic acid and melamine as the precursors. A carbon vacancy was produced by two-step calcination in argon and air atmospheres. These carbon vacancies further exposed the edges and diffusion channels of the FCN nanofibers, which accelerated photogenerated charge transfer and provided more active sites. The FCN was characterized using various techniques and used for H2 evolution under visible-light irradiation. The as-synthesized FCN exhibited excellent stability, and its photocatalytic activity for H2 evolution under visible-light irradiation was 66 times higher than that of bare C3N4 (BCN), attaining a maximum H2 evolution rate of 102.63 μmol in 6 h. The FCN remained stable following visible-light irradiation at the end of 10 cycles. The FCN benefited from the absorption of solar energy and a large number of active sites. These advantages facilitated the efficient separation of photoexcited electron-hole pairs to hinder charge recombination. This work generates new insights into the preparation of highly effective FCN photocatalysts that may be put to various applications, especially in the fields of energy and environment. Full article
(This article belongs to the Special Issue New Frontiers in Applications of Photocatalysis Processes)
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