Innovative Catalysts for Photo/Electrochemical Conversion of Small Molecules to Fuels and Value-Added Chemicals

A special issue of Catalysts (ISSN 2073-4344). This special issue belongs to the section "Environmental Catalysis".

Deadline for manuscript submissions: closed (10 December 2022) | Viewed by 2998

Special Issue Editors


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Guest Editor
Department of Colloids Chemistry, Max Planck Institute of Colloids and Interfaces, Potsdam, Germany
Interests: electrochemistry; electrocatalysis; energy conversion; energy storage; material chemistry
The Laboratory of Renewable Energy Science and Engineering, EPFL, Lausanne, Switzerland
Interests: photocatalysis; electrocatalysis; photoelectrocatalysis
Department of Chemistry, Katholieke Universiteit Leuven, Leuven, Belgium
Interests: smart poly-gel; energy storage; electrocatalysis; theoretical calculations
Institute of Analysis, Guangdong Academy of Sciences (China National Analytical Center, Guangzhou), Guangzhou, China
Interests: electrochemistry; electrocatalysis; two-dimension nanosheets

Special Issue Information

Dear Colleagues,

The emerging photo/electro-convert renewable small molecules (H2O, CO2, N2, O2, H2, NH3, CH4, etc.) of transportable fuels and value-added chemicals, as a sustainable and environmentally benign technology, are of great potential to replace the traditional fossil fuel-based industrial synthesis. The development of appropriate reaction systems and innovative catalysts is a key step in the photo/electrocatalytic process for efficient activation and formation of chemical bonds. Although recently these reactions have been well-studied, the catalyst design, system optimization and reaction mechanisms for the objective of high selectivity and yield are yet to reach their optimum in consideration of the requirement of applications.

Therefore, this Special Issue of Catalysts will highlight recent developments in the photo/electrochemical conversion of small molecules to fuels and value-added chemicals. The Guest Editors welcome submissions of original research and review articles by researchers from all disciplines investigating topics relevant to the photo/electrochemical synthesis of fuels and value-added chemicals, including, but not limited to, the following:

  • Water Splitting for H2 production;
  • CO2 reduction;
  • N2 fixation, including N2 reduction and oxidation;
  • Nitrogen oxide molecule/ion (NO, NO3-, NO2-, etc.) reduction;
  • CH4 oxidation;
  • O2 reduction;
  • H2 oxidation;
  • Integrated reactions, i. e., coupling CO2 and N2 reduction reaction.

Submit your paper and select the Journal “Catalysts” and the Special Issue “Innovative catalysts for photo/electrochemical conversion of small molecules to fuels and value-added chemicals” via MDPI submission system. Please contact the Guest Editor or the journal editor ([email protected]) for any queries. Our papers will be published on a rolling basis and we will be pleased to receive your submission once you have finished it.

Dr. Gaofeng Chen
Dr. Jian Li
Dr. Feili Lai
Dr. Hui Cheng
Guest Editors

Manuscript Submission Information

Manuscripts should be submitted online at www.mdpi.com by registering and logging in to this website. Once you are registered, click here to go to the submission form. Manuscripts can be submitted until the deadline. All submissions that pass pre-check are peer-reviewed. Accepted papers will be published continuously in the journal (as soon as accepted) and will be listed together on the special issue website. Research articles, review articles as well as short communications are invited. For planned papers, a title and short abstract (about 100 words) can be sent to the Editorial Office for announcement on this website.

Submitted manuscripts should not have been published previously, nor be under consideration for publication elsewhere (except conference proceedings papers). All manuscripts are thoroughly refereed through a single-blind peer-review process. A guide for authors and other relevant information for submission of manuscripts is available on the Instructions for Authors page. Catalysts is an international peer-reviewed open access monthly journal published by MDPI.

Please visit the Instructions for Authors page before submitting a manuscript. The Article Processing Charge (APC) for publication in this open access journal is 2700 CHF (Swiss Francs). Submitted papers should be well formatted and use good English. Authors may use MDPI's English editing service prior to publication or during author revisions.

Keywords

  • photocatalysis
  • electrocatalysis
  • small molecules
  • fuel
  • value-added chemicals
  • water splitting
  • H2 prodcution
  • CO2 reduction
  • N2 fixation
  • nitrogen oxide molecule/ion reduction
  • CH4 oxidation
  • O2 reduction
  • integrated reactions

Published Papers (1 paper)

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Research

12 pages, 3000 KiB  
Article
Facile Synthesis of Sulfate-Intercalated CoFe LDH Nanosheets Derived from Two-Dimensional ZIF-9(III) for Promoted Oxygen Evolution Reaction
by Guolei Xiao, Weibin Chen, Yaming Cai, Shifan Zhang, Di Wang and Dandan Cai
Catalysts 2022, 12(7), 688; https://0-doi-org.brum.beds.ac.uk/10.3390/catal12070688 - 23 Jun 2022
Cited by 8 | Viewed by 2348
Abstract
Layered double hydroxide (LDH) has emerged as a promising electrocatalyst; however, the synthetic method usually requires high temperature and high pressure, and sulfate-intercalated LDH is rarely reported. Herein, the sulfate-intercalated CoFe LDH nanosheets were successfully fabricated at ambient temperature via a facile strategy, [...] Read more.
Layered double hydroxide (LDH) has emerged as a promising electrocatalyst; however, the synthetic method usually requires high temperature and high pressure, and sulfate-intercalated LDH is rarely reported. Herein, the sulfate-intercalated CoFe LDH nanosheets were successfully fabricated at ambient temperature via a facile strategy, using two-dimensional ZIF-9(III) as a template and FeSO4 as both etchant and iron source. When the as-prepared sulfate-intercalated CoFe LDH acts as an electrocatalyst, it presents superior electrocatalytic performance for the oxygen evolution reaction (OER), requiring low overpotential (η@10 mA cm−2 = 218 mV) with a small Tafel slope of 59.9 mV dec−1 in 1.0 M KOH, which compares favorably with commercial RuO2 and most reported transition-metal electrocatalysts. The high catalytic activity of CoFe LDH might be ascribed to the large interlayer space distance originating from special SO42− ions and the strong synergistic effects between Fe and Co. This work provides a novel and feasible approach to designing highly efficient electrocatalysts based on advanced LDH materials for OER. Full article
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