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Linear and Non-linear AC Magnetic Susceptibility for the Study of Superconducting and Magnetic Materials

A special issue of Materials (ISSN 1996-1944). This special issue belongs to the section "Materials Physics".

Deadline for manuscript submissions: closed (20 October 2022) | Viewed by 4123

Special Issue Editors


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Guest Editor
Department of Physics “E.R. Caianiello”, University of Salerno, Via Giovanni Paolo II, 132, I-84084 Fisciano, Salerno, Italy
Interests: condensed matter physics; superconductivity; AC and DC magnetic properties; multi-harmonic AC susceptibility; vortex dynamics; magnetic materials
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Guest Editor
Department of Physics “E.R. Caianiello”, University of Salerno, Via Giovanni Paolo II, 132, I-84084 Fisciano, Salerno, Italy
Interests: superconductivity; iron-based superconductors; magnetic properties of low- and high-temperature superconductors; vortex dynamics; flux pinning properties; magnetism; magnetic measurements; magnetic materials; nanomaterials; magnetic nanoparticles
Special Issues, Collections and Topics in MDPI journals

Special Issue Information

Dear Colleagues,

The AC magnetic susceptibility (ACMS) technique is a powerful tool which makes it possible to investigate the magnetic response of a material when an AC magnetic field is applied. By changing the AC field amplitude and frequency, it is possible to probe the different magnetic behaviors and obtain information about the characteristic magnetic properties of the material. In particular, the study of superconductors by means of the ACMS technique enables researchers to determine the shielding and dissipation properties of the investigated sample by analyzing the real and imaginary part of the AC fundamental harmonic, respectively, together with other important features for applications such as critical temperature, critical current density in the AC regime, pinning properties, etc. Moreover, by analyzing the first- and third-harmonic components it is possible to study the vortex dynamics of the sample, distinguishing different dissipative regimes. Concerning magnetic materials, the ACMS technique makes it possible to study the different magnetic phase transitions of the investigated sample together with the relaxation phenomena which are correlated to the spin dynamics that very often are not recognizable with DC magnetic measurements. The features that can be studied include: the freezing temperature of the spin glass systems, which can be probed using the ACMS technique since this temperature is sensible to the AC frequency variations; the blocking temperature of magnetic nanoparticles, which can be determined by the imaginary component of the fundamental harmonic; the Curie temperature for ferromagnetic samples, which can be examined by varying the AC magnetic field amplitude and frequency, also individuating various models of magnetic interactions.

This Special Issue will be focused on the AC magnetic susceptibility technique applied to superconducting (low-temperature, high-temperature, iron-based, etc.) and magnetic (spin glass, ferro/antiferro/ferri-magnetic materials, magnetic nanoparticles, etc.) materials and will include, but not be limited to, the following topics:

  • Fundamental and third harmonic of AC magnetic susceptibility in superconducting materials;
  • Vortex dynamics and dissipative regimes in superconductors in AC magnetic field;
  • AC losses in Type-II superconductors;
  • AC amplitude and frequency dependencies of the properties of ferromagnetic and antiferromagnetic materials;
  • Magnetic phase transitions;
  • Spin glass relaxation properties;
  • Magnetic nanoparticles;
  • Blocking temperature and superparamagnetic behavior.

It is our pleasure to invite you to submit a manuscript for this Special Issue. Full papers, communications, and reviews are all welcome.

Prof. Massimiliano Polichetti
Dr. Armando Galluzzi
Guest Editors

Manuscript Submission Information

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Keywords

  • AC magnetic characterization of superconducting and magnetic materials
  • multi-harmonic AC susceptibility
  • vortex dynamics and pinning properties in AC field
  • magnetic phase transitions

Published Papers (3 papers)

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Research

14 pages, 4323 KiB  
Article
Complex AC Magnetic Susceptibility as a Tool for Exploring Nonlinear Magnetic Phenomena and Pinning Properties in Superconductors
by Krastyo Buchkov, Armando Galluzzi, Elena Nazarova and Massimiliano Polichetti
Materials 2023, 16(14), 4896; https://0-doi-org.brum.beds.ac.uk/10.3390/ma16144896 - 08 Jul 2023
Cited by 3 | Viewed by 1396
Abstract
The versatile AC magnetic susceptibility technique offers a detailed insight into the complex electrodynamic phenomena in superconductors. In the present study, we outline the key effects related to the temperature, AC field amplitude and frequency variations of the fundamental and harmonic components for [...] Read more.
The versatile AC magnetic susceptibility technique offers a detailed insight into the complex electrodynamic phenomena in superconductors. In the present study, we outline the key effects related to the temperature, AC field amplitude and frequency variations of the fundamental and harmonic components for an investigation of the vortex dynamics in a flux-grown FeSe crystal. By means of higher harmonic (nonlinear) analysis, we have explored certain atypical, asymmetric features in the AC magnetic response. These effects were identified through the detection of an even (second) harmonic and an unusual temperature shift in the odd (third) harmonic, possibly due to the complex interactions related to the composite superconducting/magnetic morphology of the crystal. Using the high-frequency sensitivity of the third harmonic, the basic functional dependencies of the pinning activation energy, as the main mixed state parameter, were determined with the implementation of the Kim–Anderson Arrhenius relation in the framework of the collective creep theory. Full article
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11 pages, 1231 KiB  
Article
The Effect of a DC Magnetic Field on the AC Magnetic Properties of Oleic Acid-Coated Fe3O4 Nanoparticles
by Michele Modestino, Armando Galluzzi, Maria Sarno and Massimiliano Polichetti
Materials 2023, 16(12), 4246; https://0-doi-org.brum.beds.ac.uk/10.3390/ma16124246 - 08 Jun 2023
Cited by 4 | Viewed by 943
Abstract
The AC magnetic properties of a sample of Fe3O4 nanoparticles coated with oleic acid have been investigated with the help of AC susceptibility measurements. In particular, several DC magnetic fields have been superimposed on the AC field, and their effect [...] Read more.
The AC magnetic properties of a sample of Fe3O4 nanoparticles coated with oleic acid have been investigated with the help of AC susceptibility measurements. In particular, several DC magnetic fields have been superimposed on the AC field, and their effect on the magnetic response of the sample has been analysed. The results show the presence of a double peak structure in the imaginary component of the complex AC susceptibility measured as a function of the temperature. A preliminary evaluation of the Mydosh parameter for both peaks gives the information that each one of them is associated with a different state of interaction between nanoparticles. The two peaks evolve both in amplitude and position when the intensity of the DC field is changed. The field dependence of the peak position shows two different trends, and it is possible to study them in the framework of the currently existing theoretical models. In particular, a model of non-interacting magnetic nanoparticles has been used to describe the behaviour of the peak at lower temperatures, whereas the behaviour of the peak at higher temperatures has been analysed in the framework of a spin-glass-like model. The proposed analysis technique can be useful for the characterisation of magnetic nanoparticles used in several types of applications, such as biomedical and magnetic fluids. Full article
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12 pages, 4123 KiB  
Article
High-Frequency ac Susceptibility of Iron-Based Superconductors
by Gianluca Ghigo, Michela Fracasso, Roberto Gerbaldo, Laura Gozzelino, Francesco Laviano, Andrea Napolitano, Guang-Han Cao, Michael J. Graf, Ruslan Prozorov, Tsuyoshi Tamegai, Zhixiang Shi, Xiangzhuo Xing and Daniele Torsello
Materials 2022, 15(3), 1079; https://0-doi-org.brum.beds.ac.uk/10.3390/ma15031079 - 29 Jan 2022
Cited by 4 | Viewed by 2332
Abstract
A microwave technique suitable for investigating the AC magnetic susceptibility of small samples in the GHz frequency range is presented. The method—which is based on the use of a coplanar waveguide resonator, within the resonator perturbation approach—allows one to obtain the absolute value [...] Read more.
A microwave technique suitable for investigating the AC magnetic susceptibility of small samples in the GHz frequency range is presented. The method—which is based on the use of a coplanar waveguide resonator, within the resonator perturbation approach—allows one to obtain the absolute value of the complex susceptibility, from which the penetration depth and the superfluid density can be determined. We report on the characterization of several iron-based superconducting systems, belonging to the 11, 122, 1144, and 12442 families. In particular, we show the effect of different kinds of doping for the 122 family, and the effect of proton irradiation in a 122 compound. Finally, the paradigmatic case of the magnetic superconductor EuP-122 is discussed, since it shows the emergence of both superconducting and ferromagnetic transitions, marked by clear features in both the real and imaginary parts of the AC susceptibility. Full article
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