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Nanomaterials
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Novel Ways of Developing Bio- and Electrochemical Sensors with Nanomaterials
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Novel Ways of Developing Bio- and Electrochemical Sensors with Nanomaterials

A special issue of Nanomaterials (ISSN 2079-4991). This special issue belongs to the section "Nanoelectronics, Nanosensors and Devices".

Deadline for manuscript submissions: 10 May 2024 | Viewed by 2123

Special Issue Editor

Dr. Seong Jung Kwon

E-Mail Website
Guest Editor
Department of Chemistry, Konkuk University, Seoul, Republic of Korea
Interests: single nanoparticle electrochemistry; electrochemical biosensor; electrochemical reaction for energy
Special Issues, Collections and Topics in MDPI journals

Special Issue Information

Dear Colleagues,

This Special Issue will center its attention on the comprehensive exploration of electrochemical sensing and nano biosensing strategies employing advanced nanomaterials. We invite submissions encompassing, but not limited to, the following areas:

  • Advancements in electrocatalytic functionalization and signal amplification harnessing a diverse array of nanomaterials, including metal nanoparticles, semiconductor nanoparticles, carbon-based nanomaterials, nanowires, liposomes, and silica nanoparticles;
  • Explorations into localized electrochemistry at the nanometer scale, encompassing the fabrication and characterization of nanoelectrodes, electrochemical investigations of collisions between nanomaterials and electrodes, electrochemistry of immobilized single nanomaterials, as well as electrochemistry within nanopipettes and redox cycling within nanopores;
  • In-depth investigations into the physics and chemistry of sensor and actuator materials, involving the development and characterization of novel compositions utilizing nanomaterials;

Pioneering concepts, designs, modeling, and validation of innovative sensor and actuator technologies, along with the integration of nanomaterials to enhance functionality and performance

Dr. Seong Jung Kwon
Guest Editor

Manuscript Submission Information

Manuscripts should be submitted online at www.mdpi.com by registering and logging in to this website. Once you are registered, click here to go to the submission form. Manuscripts can be submitted until the deadline. All submissions that pass pre-check are peer-reviewed. Accepted papers will be published continuously in the journal (as soon as accepted) and will be listed together on the special issue website. Research articles, review articles as well as short communications are invited. For planned papers, a title and short abstract (about 100 words) can be sent to the Editorial Office for announcement on this website.

Submitted manuscripts should not have been published previously, nor be under consideration for publication elsewhere (except conference proceedings papers). All manuscripts are thoroughly refereed through a single-blind peer-review process. A guide for authors and other relevant information for submission of manuscripts is available on the Instructions for Authors page. Nanomaterials is an international peer-reviewed open access semimonthly journal published by MDPI.

Please visit the Instructions for Authors page before submitting a manuscript. The Article Processing Charge (APC) for publication in this open access journal is 2900 CHF (Swiss Francs). Submitted papers should be well formatted and use good English. Authors may use MDPI's English editing service prior to publication or during author revisions.

Keywords

  • electrochemistry
  • biosensor
  • nanoparticle
  • nanomaterial
  • electrochemical reaction for energy
  • nanocomposites
  • microsensor
  • diagnostic
  • cell

Published Papers (3 papers)

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Research

17 pages, 4488 KiB  
Article
Highly Sensitive Electrochemical Determination of Butylated Hydroxyanisole in Food Samples Using Electrochemical-Pretreated Three-Dimensional Graphene Electrode Modified with Silica Nanochannel Film
by Chengqing Huang, Shiyue Zhang, Xinying Ma, Fei Yan and Weizhong Tang
Nanomaterials 2024, 14(7), 569; https://0-doi-org.brum.beds.ac.uk/10.3390/nano14070569 - 25 Mar 2024
Viewed by 611
Abstract
The sensitive detection of antioxidants in food is essential for the rational control of their usage and reducing potential health risks. A simple three-dimensional (3D) electrode integrated with an anti-fouling/anti-interference layer possesses great potential for the direct and sensitive electrochemical detection of antioxidants [...] Read more.
The sensitive detection of antioxidants in food is essential for the rational control of their usage and reducing potential health risks. A simple three-dimensional (3D) electrode integrated with an anti-fouling/anti-interference layer possesses great potential for the direct and sensitive electrochemical detection of antioxidants in food samples. In this work, a 3D electrochemical sensor was developed by integrating a 3D graphene electrode (3DG) with vertically ordered mesoporous silica film (VMSF), enabling highly sensitive detection of the common antioxidant, butylated hydroxyanisole (BHA), in food samples. A simple electrochemical polarization was employed to pre-activate the 3DG electrode (p3DG), enhancing its hydrophilicity. Using the p3DG as the supporting electrode, stable modification of VMSF was achieved using the electrochemical assisted self-assembly (EASA) method, without the need for any adhesive agents (VMSF/p3DG). Taking BHA in food as a model analyte, the VMSF/p3DG sensor demonstrated high sensitivity, due to the enrichment by nanochannels, towards BHA. Electrochemical detection of BHA was achieved with a linear range of 0.1 μM to 5 μM and from 5 μM to 150 μM with a low limit of detection (12 nM). Owing to the fouling resistance and anti-interference capabilities of VMSF, the constructed 3D electrochemical sensor can be directly applied for the electrochemical detection of BHA in complex food samples. Full article
(This article belongs to the Special Issue Novel Ways of Developing Bio- and Electrochemical Sensors with Nanomaterials)
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11 pages, 3305 KiB  
Article
Highly Sensitive and Stable Multifunctional Self-Powered Triboelectric Sensor Utilizing Mo2CTx/PDMS Composite Film for Pressure Sensing and Non-Contact Sensing
by Jialiang Fan, Chenxing Wang, Bo Wang, Bin Wang and Fangmeng Liu
Nanomaterials 2024, 14(5), 428; https://0-doi-org.brum.beds.ac.uk/10.3390/nano14050428 - 27 Feb 2024
Viewed by 643
Abstract
Sensors based on triboelectric nanogenerators (TENGs) are increasingly gaining attention because of their self-powered capabilities and excellent sensing performance. In this work, we report a Mo2CTx-based triboelectric sensor (Mo-TES) consisting of a Mo2CTx/polydimethylsiloxane (PDMS) composite [...] Read more.
Sensors based on triboelectric nanogenerators (TENGs) are increasingly gaining attention because of their self-powered capabilities and excellent sensing performance. In this work, we report a Mo2CTx-based triboelectric sensor (Mo-TES) consisting of a Mo2CTx/polydimethylsiloxane (PDMS) composite film. The impact of the mass fraction (wt%) and force of Mo2CTx particles on the output performance of Mo-TES was systematically explored. When Mo2CTx particles is 3 wt%, Mo-TES3 achieves an open-circuit voltage of 86.89 V, a short-circuit current of 578.12 nA, and a power density of 12.45 μW/cm2. It also demonstrates the ability to charge capacitors with varying capacitance values. Additionally, the Mo-TES3 demonstrates greater sensitivity than the Mo-TES0 and a faster recovery time of 78 ms. Meanwhile, the Mo-TES3 also demonstrates excellent stability in water washing and antifatigue testing. This demonstrates the effectiveness of Mo-TES as a pressure sensor. Furthermore, leveraging the principle of electrostatic induction, the triboelectric sensor has the potential to achieve non-contact sensing, making it a promising candidate for disease prevention and safety protection. Full article
(This article belongs to the Special Issue Novel Ways of Developing Bio- and Electrochemical Sensors with Nanomaterials)
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15 pages, 4190 KiB  
Article
Solid Electrochemiluminescence Sensor by Immobilization of Emitter Ruthenium(II)tris(bipyridine) in Bipolar Silica Nanochannel Film for Sensitive Detection of Oxalate in Serum and Urine
by Ruliang Yu, Yujiao Zhao and Jiyang Liu
Nanomaterials 2024, 14(5), 390; https://0-doi-org.brum.beds.ac.uk/10.3390/nano14050390 - 20 Feb 2024
Cited by 3 | Viewed by 701
Abstract
Convenient and highly sensitive detection of oxalate ions in body fluids is of crucial significance for disease prevention, diagnosis, and monitoring of treatment effectiveness. Establishing a simple solid-state electrochemiluminescence (ECL) sensing system for highly sensitive detection of oxalate ions is highly desirable. In [...] Read more.
Convenient and highly sensitive detection of oxalate ions in body fluids is of crucial significance for disease prevention, diagnosis, and monitoring of treatment effectiveness. Establishing a simple solid-state electrochemiluminescence (ECL) sensing system for highly sensitive detection of oxalate ions is highly desirable. In this work, a solid ECL sensor was fabricated by immobilizing the commonly used emitter ruthenium(II)tris(bipyridine) (Ru(bpy)32+) on a double-layered bipolar silica nanochannel array film (bp-SNA)-modified electrode, enabling sensitive detection of oxalate ions in serum or urine samples. Cost-effective and readily available indium tin oxide (ITO) was used as the supporting electrode. Convenient fabrication of multiple negatively charged SNA (n-SNA)-modified ITO electrodes was achieved through the one-step Stöber solution growth method. Subsequently, a positive outer layer film (p-SNA) was rapidly prepared using an electrochemical-assisted self-assembly method. The double-layered bipolar silica nanochannel array film achieved stable immobilization of Ru(bpy)32+ on the electrode surface, facilitated by the electrostatic adsorption of Ru(bpy)32+ by n-SNA and the electrostatic repulsion by p-SNA. Utilizing oxalate ions as a co-reactant for Ru(bpy)32+, combined with the electrostatic enrichment of oxalate ions by p-SNA, the constructed sensor enabled highly sensitive detection of oxalate ions ranging from 1 nM to 25 μM and from 25 μM to 1 mM, with a detection limit (LOD) of 0.8 nM. The fabricated ECL sensor exhibited high selectivity and good stability, making it suitable for ECL detection of oxalate ions in serum and urine samples. Full article
(This article belongs to the Special Issue Novel Ways of Developing Bio- and Electrochemical Sensors with Nanomaterials)
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