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Applied Sciences
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High Capacity Electrode Materials for Advanced Lithium Ion Batteries
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High Capacity Electrode Materials for Advanced Lithium Ion Batteries

A special issue of Applied Sciences (ISSN 2076-3417). This special issue belongs to the section "Materials Science and Engineering".

Deadline for manuscript submissions: closed (31 July 2019) | Viewed by 18541

Special Issue Editor

Dr. Gaind P. Pandey

E-Mail Website
Guest Editor
Giner Inc., Newton, MA 02466, USA
Interests: energy storage; supercapacitors; lithium-ion batteries; alloying anodes; si-c anodes; lithium-sulfur batteries; polymer electrolytes; polymer-ceramic (hybrid) electrolytes; ionic liquids; ionogels

Special Issue Information

Dear Colleagues,

With the ever-growing applications of the lithium-ion battery (LIB), from consumer electronics to electric vehicles, the demand for Li-ion batteries with increased energy density is more urgent than ever before. High energy density LIBs need both anode and cathode materials with high capacities for hosting Li-ions. In response to this demand, considerable research efforts have been directed toward improving the energy density of batteries by developing high-capacity electrode materials such as Li-rich (or Li-excess) cathodes, Ni-rich cathodes, and Si anodes, and other high-capacity anode and cathode materials. High-capacity anode research, in particular, has been active, and materials such as silicon (Si), tin (Sn), germanium (Ge) and tin oxides (SnOx) have received significant attention. To address the most state-of-the-art in the research and development of high capacity electrodes (both anode and cathode) for lithium-ion batteries, in this Special Issue, we invite research, review articles, and perspectives. The contents of the manuscripts will include, but are not limited to, the following topics:

  • High capacity cathode materials for lithium-ion batteries
  • High capacity anode materials for lithium-ion batteries
  • Alloying anode (e.g., Si. Sn, Ge, etc.)
  • New design and concept for high capacity electrodes
  • Methods for performance analysis and material characterization
  • Various cell design with different combination of anode and cathode.

Dr. Gaind P. Pandey
Guest Editor

Manuscript Submission Information

Manuscripts should be submitted online at www.mdpi.com by registering and logging in to this website. Once you are registered, click here to go to the submission form. Manuscripts can be submitted until the deadline. All submissions that pass pre-check are peer-reviewed. Accepted papers will be published continuously in the journal (as soon as accepted) and will be listed together on the special issue website. Research articles, review articles as well as short communications are invited. For planned papers, a title and short abstract (about 100 words) can be sent to the Editorial Office for announcement on this website.

Submitted manuscripts should not have been published previously, nor be under consideration for publication elsewhere (except conference proceedings papers). All manuscripts are thoroughly refereed through a single-blind peer-review process. A guide for authors and other relevant information for submission of manuscripts is available on the Instructions for Authors page. Applied Sciences is an international peer-reviewed open access semimonthly journal published by MDPI.

Please visit the Instructions for Authors page before submitting a manuscript. The Article Processing Charge (APC) for publication in this open access journal is 2400 CHF (Swiss Francs). Submitted papers should be well formatted and use good English. Authors may use MDPI's English editing service prior to publication or during author revisions.

Keywords

  • Alloying materials (e.g. Si, Ge, Sn etc.)
  • Si-C composite anodes
  • Nickel-rich layered oxides (LiNi1-xMxO2, M = Co, Mn and Al),
  • Lithium-rich layered oxides (Li1+xM1-xO2, M = Mn, Ni, Co, etc.),
  • High-voltage spinel oxides (LiNi0.5Mn1.5O4)
  • High-voltage polyanionic compounds (phosphates, sulfates, silicates, etc.)

Published Papers (3 papers)

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Research

17 pages, 6690 KiB  
Article
Centrifugally Spun α-Fe2O3/TiO2/Carbon Composite Fibers as Anode Materials for Lithium-Ion Batteries
by Luis Zuniga, Gabriel Gonzalez, Roberto Orrostieta Chavez, Jason C. Myers, Timothy P. Lodge and Mataz Alcoutlabi
Appl. Sci. 2019, 9(19), 4032; https://0-doi-org.brum.beds.ac.uk/10.3390/app9194032 - 26 Sep 2019
Cited by 25 | Viewed by 3520
Abstract
We report results on the electrochemical performance of flexible and binder-free α-Fe2O3/TiO2/carbon composite fiber anodes for lithium-ion batteries (LIBs). The composite fibers were produced via centrifugal spinning and subsequent thermal processing. The fibers were prepared from a [...] Read more.
We report results on the electrochemical performance of flexible and binder-free α-Fe2O3/TiO2/carbon composite fiber anodes for lithium-ion batteries (LIBs). The composite fibers were produced via centrifugal spinning and subsequent thermal processing. The fibers were prepared from a precursor solution containing PVP/iron (III) acetylacetonate/titanium (IV) butoxide/ethanol/acetic acid followed by oxidation at 200 °C in air and then carbonization at 550 °C under flowing argon. The morphology and structure of the composite fibers were characterized using X-ray diffraction (XRD), scanning electron microscopy (SEM), transmission electron microscopy (TEM), energy dispersive X-ray spectroscopy (EDS), X-ray photoelectron spectroscopy (XPS), and thermogravimetric analysis (TGA). These ternary composite fiber anodes showed an improved electrochemical performance compared to the pristine TiO2/C and α-Fe2O3/C composite fiber electrodes. The α-Fe2O3/TiO2/C composite fibers also showed a superior cycling performance with a specific capacity of 340 mAh g−1 after 100 cycles at a current density of 100 mA g−1, compared to 61 mAh g−1 and 121 mAh g−1 for TiO2/C and α-Fe2O3/C composite electrodes, respectively. The improved electrochemical performance and the simple processing of these metal oxide/carbon composite fibers make them promising candidates for the next generation and cost-effective flexible binder-free anodes for LIBs. Full article
(This article belongs to the Special Issue High Capacity Electrode Materials for Advanced Lithium Ion Batteries)
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16 pages, 9347 KiB  
Article
The Effect of Compactness on Laser Cutting of Cathode for Lithium-Ion Batteries Using Continuous Fiber Laser
by Dongkyoung Lee, Byungmoon Oh and Jungdon Suk
Appl. Sci. 2019, 9(1), 205; https://0-doi-org.brum.beds.ac.uk/10.3390/app9010205 - 08 Jan 2019
Cited by 14 | Viewed by 8138
Abstract
Lithium-Ion Batteries (LIB) are growing in popularity for many applications. Much research has been focusing on battery performance improvement. However, few studies have overcome the disadvantages of the conventional LIB manufacturing processes. Laser cutting of electrodes has been applied. However, the effect of [...] Read more.
Lithium-Ion Batteries (LIB) are growing in popularity for many applications. Much research has been focusing on battery performance improvement. However, few studies have overcome the disadvantages of the conventional LIB manufacturing processes. Laser cutting of electrodes has been applied. However, the effect of electrodes’ chemical, physical, and geometrical characteristics on the laser cutting has not been considered. This study proposes the effect of compression of cathode on laser cutting for lithium-ion batteries. The kerf width and top width of the specimens with laser irradiation are measured and the material removal energy is obtained. Observations of SEM photographs and absorptivity measurements are conducted. Increasing volume energies causes logarithmic increases in the kerf and top width. It is observed that the compressed cathode forms a wider kerf width than the uncompressed cathode under the same laser parameters. The top width of the uncompressed cathode is wider than the uncompressed cathode. The compression has a favorable effect on uniform cutting and selective removal of an active electrode. Full article
(This article belongs to the Special Issue High Capacity Electrode Materials for Advanced Lithium Ion Batteries)
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9 pages, 3193 KiB  
Article
Systematic Investigation of Prelithiated SiO2 Particles for High-Performance Anodes in Lithium-Ion Battery
by Yuyao Han, Xinyi Liu and Zhenda Lu
Appl. Sci. 2018, 8(8), 1245; https://0-doi-org.brum.beds.ac.uk/10.3390/app8081245 - 27 Jul 2018
Cited by 28 | Viewed by 6256
Abstract
Prelithiation is an important strategy used to compensate for lithium loss during the formation of a solid electrolyte interface (SEI) layer and the other irreversible reactions at the first stage of electrochemical cycling. In this paper, we report a systematic study of thermal [...] Read more.
Prelithiation is an important strategy used to compensate for lithium loss during the formation of a solid electrolyte interface (SEI) layer and the other irreversible reactions at the first stage of electrochemical cycling. In this paper, we report a systematic study of thermal prelithiation of SiO2 particles with different sizes (6 nm, 20 nm, 300 nm and 3 μm). All four lithiated anodes (LixSi/Li2O composites) show improved performance over pristine SiO2. More interestingly, lithiated product from micron-sized SiO2 particle demonstrates optimum performance with a charge capacity of 1859 mAhg−1 initially and maintains above 1300 mAhg−1 for over 50 cycles. Full article
(This article belongs to the Special Issue High Capacity Electrode Materials for Advanced Lithium Ion Batteries)
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